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  1. 040 理学部
  2. 0401 学術論文

Synthesis of donor-acceptor chromophores by the [2+2] cycloaddition of arylethynyl-2H-cyclohepta[b]furan-2-ones with 7,7,8,8-tetracyanoquinodimethane

http://hdl.handle.net/10091/16091
http://hdl.handle.net/10091/16091
8f47cf0e-a786-4bc1-9506-b8ba20853639
名前 / ファイル ライセンス アクション
Org. Org. Biomol. Chem., 2012, 10, 2431.pdf (548.6 kB)
Item type 学術雑誌論文 / Journal Article(1)
公開日 2012-11-26
タイトル
言語 en
タイトル Synthesis of donor-acceptor chromophores by the [2+2] cycloaddition of arylethynyl-2H-cyclohepta[b]furan-2-ones with 7,7,8,8-tetracyanoquinodimethane
言語
言語 eng
資源タイプ
資源 http://purl.org/coar/resource_type/c_6501
タイプ journal article
著者 Shoji, Taku

× Shoji, Taku

WEKO 36227

Shoji, Taku

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Higashi, Junya

× Higashi, Junya

WEKO 36228

Higashi, Junya

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Ito, Shunji

× Ito, Shunji

WEKO 36229

Ito, Shunji

Search repository
Okujima, Tetsuo

× Okujima, Tetsuo

WEKO 36230

Okujima, Tetsuo

Search repository
Yasunami, Masafumi

× Yasunami, Masafumi

WEKO 36231

Yasunami, Masafumi

Search repository
Morita, Noboru

× Morita, Noboru

WEKO 36232

Morita, Noboru

Search repository
信州大学研究者総覧へのリンク
氏名 Shoji, Taku
URL http://soar-rd.shinshu-u.ac.jp/profile/ja.gmShOakh.html
出版者
出版者 ROYAL SOC CHEMISTRY
引用
内容記述タイプ Other
内容記述 ORGANIC & BIOMOLECULAR CHEMISTRY. 10(12):2431-2438 (2012)
書誌情報 ORGANIC & BIOMOLECULAR CHEMISTRY

巻 10, 号 12, p. 2431-2438, 発行日 2012
抄録
内容記述タイプ Abstract
内容記述 Arylethynyl-2H-cyclohepta[b]furan-2-ones reacted with 7,7,8,8-tetracyanoquinodimethane (TCNQ) in a formal [2 + 2] cycloaddition reaction, followed by ring opening of the initially formed cyclobutene derivatives, to afford the corresponding dicyanoquinodimethane (DCNQ) chromophores in excellent yields. The intramolecular charge-transfer (ICT) interactions between the 2H-cyclohepta[b]furan-2-one ring and DCNQ acceptor moiety were investigated by UV/Vis spectroscopy and theoretical calculations. The redox behavior of the novel DCNQ derivatives was examined by cyclic voltammetry (CV) and differential pulse voltammetry (DPV), which revealed their multistep electrochemical reduction properties depended on the number of DCNQ units in the molecule. Moreover, a significant color change was observed by visible spectroscopy under electrochemical reduction conditions.
資源タイプ(コンテンツの種類)
内容記述タイプ Other
内容記述 Article
ISSN
収録物識別子タイプ ISSN
収録物識別子 1477-0520
書誌レコードID
収録物識別子タイプ NCID
収録物識別子 AA1168650X
PubMed
識別子タイプ PMID
関連識別子 http://www.ncbi.nlm.nih.gov/entrez/query.fcgi?CMD=search&DB=pubmed&term=22331190
関連名称 22331190
DOI
識別子タイプ DOI
関連識別子 https://doi.org/10.1039/c2ob06931h
関連名称 10.1039/c2ob06931h
権利
権利情報 Org. Biomol. Chem., 2012,10, 2431-2438 - Reproduced by permission of The Royal Society of Chemistry
出版タイプ
出版タイプ AM
出版タイプResource http://purl.org/coar/version/c_ab4af688f83e57aa
WoS
表示名 Web of Science
URL http://gateway.isiknowledge.com/gateway/Gateway.cgi?&GWVersion=2&SrcAuth=ShinshuUniv&SrcApp=ShinshuUniv&DestLinkType=FullRecord&DestApp=WOS&KeyUT=000301058100015
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