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When H(2)A was co-existent in a Ru(bpy)(3)(2+)-containing buffer solution, ECL peaks were observed at a potential corresponding to the oxidation of Ru(bpy)(3)(2+), and the intensity was proportional to H(2)A concentration at lower concentration levels. The formation of the excited state *Ru(bpy)(3)(2+) was confirmed to result from the co-reaction between Ru(bpy)(3)(2+) and the intermediate of ascorbate anion radical (A(-)center dot), which showed the maximum ECL at pH = 8.8. It is our first finding that the ECL intensity would be quenched significantly when the concentration of H(2)A was relatively higher, or upon ultrasonic irradiation. In most instances, quenching is observed with four-fold excess of H(2)A over Ru(bpy)(3)(2+). The diffusional self-quenching scheme as well as the possible reaction pathways involved in the Ru(bpy)(3)(2+)-H(2)A ECL system are discussed in this study. 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  1. 040 理学部
  2. 0401 学術論文

Self-quenching in the electrochemiluminescence of Ru(bpy)(3)(2+) using ascorbic acid as co-reactant

http://hdl.handle.net/10091/1136
da320886-9814-436a-81aa-b08121c08825
名前 / ファイル ライセンス アクション
Manuscript_Luminescence_revised[1].pdf Manuscript_Luminescence_revised[1].pdf (334.1 kB)
Item type 学術雑誌論文 / Journal Article(1)
公開日 2008-09-08
タイトル
言語 en
タイトル Self-quenching in the electrochemiluminescence of Ru(bpy)(3)(2+) using ascorbic acid as co-reactant
言語
言語 eng
資源タイプ
資源 http://purl.org/coar/resource_type/c_6501
タイプ journal article
著者 Takahashi, F

× Takahashi, F

WEKO 36664

Takahashi, F

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Jin, JY

× Jin, JY

WEKO 36665

Jin, JY

Search repository
信州大学研究者総覧へのリンク
氏名 Jin, JY
URL http://soar-rd.shinshu-u.ac.jp/profile/ja.jUThymkV.html
出版者
出版者 JOHN WILEY & SONS LTD
引用
内容記述タイプ Other
内容記述 LUMINESCENCE. 23(3):121-125(2008)
書誌情報 LUMINESCENCE

巻 23, 号 3, p. 121-125, 発行日 2008-05
資源タイプ(コンテンツの種類)
内容記述タイプ Other
内容記述 Article
ISSN
収録物識別子タイプ ISSN
収録物識別子 1522-7235
書誌レコードID
収録物識別子タイプ NCID
収録物識別子 AA00701292
DOI
関連識別子
識別子タイプ DOI
関連識別子 https://doi.org/10.1002/bio.1019
関連名称
関連名称 10.1002/bio.1019
出版タイプ
出版タイプ AM
出版タイプResource http://purl.org/coar/version/c_ab4af688f83e57aa
WoS
表示名 Web of Science
URL http://gateway.isiknowledge.com/gateway/Gateway.cgi?&GWVersion=2&SrcAuth=ShinshuUniv&SrcApp=ShinshuUniv&DestLinkType=FullRecord&DestApp=WOS&KeyUT=000257828700002
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