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H-1 NMR spectra of 4 and 5 exhibited an unequal shielding effect on the bridge hydrogens from the resulted it ring system, suggesting the existence of the significant homoconjugative transannular interaction on the nonadjacent carbons at the bridge and the discreteness of pi-conjugation of the annulene between two bonds at the C7-C8 and C11-C12 to localize the C8-11 dienyl and the remaining parts. The X-ray crystallographic structures of 4 and 5 show relatively short atomic distance between those bridge carbons, and clear bond alternation of the dienyl part and the bond convergence of the remaining part in these compounds, supporting the spectral properties. (C) 2007 Elsevier Ltd. 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  1. 040 理学部
  2. 0401 学術論文

Discreteness of pi-conjugation of 1,6-methano[10]annulene by troponoid fusion at the 3,4-positions

http://hdl.handle.net/10091/1059
http://hdl.handle.net/10091/1059
3fde4b8b-f4e8-4549-b44c-672d2ae059af
名前 / ファイル ライセンス アクション
小田 小田 晃規 TL_888_2008.pdf (122.7 kB)
Item type 学術雑誌論文 / Journal Article(1)
公開日 2008-05-30
タイトル
言語 en
タイトル Discreteness of pi-conjugation of 1,6-methano[10]annulene by troponoid fusion at the 3,4-positions
言語
言語 eng
資源タイプ
資源 http://purl.org/coar/resource_type/c_6501
タイプ journal article
著者 Zhang, YM

× Zhang, YM

WEKO 36695

Zhang, YM

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Hisano, E

× Hisano, E

WEKO 36696

Hisano, E

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Ohta, R

× Ohta, R

WEKO 36697

Ohta, R

Search repository
Miyatake, R

× Miyatake, R

WEKO 36698

Miyatake, R

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Horino, Y

× Horino, Y

WEKO 36699

Horino, Y

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Oda, M

× Oda, M

WEKO 36700

Oda, M

Search repository
Kuroda, S

× Kuroda, S

WEKO 36701

Kuroda, S

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信州大学研究者総覧へのリンク
氏名 Oda, M
URL http://soar-rd.shinshu-u.ac.jp/profile/ja.gNAmbVkm.html
出版者
出版者 PERGAMON-ELSEVIER SCIENCE LTD
引用
内容記述タイプ Other
内容記述 TETRAHEDRON LETTERS. 49(5): 888-892 (2008)
書誌情報 TETRAHEDRON LETTERS

巻 49, 号 5, p. 888-892, 発行日 2008-01-28
資源タイプ(コンテンツの種類)
内容記述タイプ Other
内容記述 Article
ISSN
収録物識別子タイプ ISSN
収録物識別子 0040-4039
書誌レコードID
収録物識別子タイプ NCID
収録物識別子 AA00861801
DOI
識別子タイプ DOI
関連識別子 https://doi.org/10.1016/j.tetlet.2007.11.161
関連名称 10.1016/j.tetlet.2007.11.161
出版タイプ
出版タイプ AM
出版タイプResource http://purl.org/coar/version/c_ab4af688f83e57aa
WoS
表示名 Web of Science
URL http://gateway.isiknowledge.com/gateway/Gateway.cgi?&GWVersion=2&SrcAuth=ShinshuUniv&SrcApp=ShinshuUniv&DestLinkType=FullRecord&DestApp=WOS&KeyUT=000253170200036
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