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The cyt c adsorbed on the modified gold electrode exhibited well-defined reversible electrochemical behavior in 10 mM phosphate buffer solution (PBS, pH 7.0). The surface concentration (F) of electroactive species, cyt c, on the binary SAMs was higher than that in single-component SAMs of T-COOH, and reached a maximum value of 9.2 x 10(-12) mol cm(-2) when the ratio of T-COOH to T-NH2 in adsorption solution was of 3:2, and the formal potential (E-0\u0027 = (E-pa + E-pc)/2) of cyt c was -0.032 V (vs. Ag vertical bar AgCl (3 M NaCl)) in a 10 mM PBS. The interaction between cyt c and the binary SAMs made the E-0\u0027 shift negatively when compared with that of cyt c in solution (+0.258 V vs. NHE, i.e., +0.058 V vs. Ag vertical bar AgCl (3 M NaCl)). The fractional coverage of bound cyt c was a 0.64 theoretical monolayer. The standard electron transfer rate constant of cyt c immobilized on the binary SAMs was also higher than that on single-component SAMs of T-COOH, and the maximum value of 15.8 +/- 0.6 s(-1) was obtained when the ratio of T-COOH to T-NH2 in adsorption solution was at 3:2. The results suggest that the electrode modified with the binary SAMs functions better than the electrode modified with single-component SAMs of T-COOH. (c) 2006 Elsevier B.V. All rights reserved."}]}, "item_creator": {"attribute_name": "著者", "attribute_type": "creator", "attribute_value_mlt": [{"creatorNames": [{"creatorName": "Ji, XP"}], "nameIdentifiers": [{"nameIdentifier": "36792", "nameIdentifierScheme": "WEKO"}]}, {"creatorNames": [{"creatorName": "Jin, BK"}], "nameIdentifiers": [{"nameIdentifier": "36793", "nameIdentifierScheme": "WEKO"}]}, {"creatorNames": [{"creatorName": "Jin, JY"}], "nameIdentifiers": [{"nameIdentifier": "36794", "nameIdentifierScheme": "WEKO"}]}, {"creatorNames": [{"creatorName": "Nakamura, T"}], "nameIdentifiers": [{"nameIdentifier": "36795", "nameIdentifierScheme": "WEKO"}]}]}, "item_files": {"attribute_name": "ファイル情報", "attribute_type": "file", "attribute_value_mlt": [{"accessrole": "open_date", "date": [{"dateType": "Available", "dateValue": "2015-09-28"}], "displaytype": "detail", "download_preview_message": "", "file_order": 0, "filename": "Immobilized_Cytochrome_c.pdf", "filesize": [{"value": "486.1 kB"}], "format": "application/pdf", "future_date_message": "", "is_thumbnail": false, "licensetype": "license_note", "mimetype": "application/pdf", "size": 486100.0, "url": {"label": "Immobilized_Cytochrome_c.pdf", "url": "https://soar-ir.repo.nii.ac.jp/record/11996/files/Immobilized_Cytochrome_c.pdf"}, "version_id": "7615b928-b561-4278-a440-62ff76073b2e"}]}, "item_language": {"attribute_name": "言語", "attribute_value_mlt": [{"subitem_language": "eng"}]}, "item_resource_type": {"attribute_name": "資源タイプ", "attribute_value_mlt": [{"resourcetype": "journal article", "resourceuri": "http://purl.org/coar/resource_type/c_6501"}]}, "item_title": "Voltammetry of immobilized cytochrome c on novel binary self-assembled monolayers of thioctic acid and thioctic amide modified gold electrodes", "item_titles": {"attribute_name": "タイトル", "attribute_value_mlt": [{"subitem_title": "Voltammetry of immobilized cytochrome c on novel binary self-assembled monolayers of thioctic acid and thioctic amide modified gold electrodes", "subitem_title_language": "en"}]}, "item_type_id": "6", "owner": "1", "path": ["1170"], "permalink_uri": "http://hdl.handle.net/10091/175", "pubdate": {"attribute_name": "PubDate", "attribute_value": "2007-04-20"}, "publish_date": "2007-04-20", "publish_status": "0", "recid": "11996", "relation": {}, "relation_version_is_last": true, "title": ["Voltammetry of immobilized cytochrome c on novel binary self-assembled monolayers of thioctic acid and thioctic amide modified gold electrodes"], "weko_shared_id": -1}
Voltammetry of immobilized cytochrome c on novel binary self-assembled monolayers of thioctic acid and thioctic amide modified gold electrodes
http://hdl.handle.net/10091/175
http://hdl.handle.net/10091/175f52282a0-d1a0-4a9d-9d71-1ce3f2bf81b9
名前 / ファイル | ライセンス | アクション |
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Item type | 学術雑誌論文 / Journal Article(1) | |||||
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公開日 | 2007-04-20 | |||||
タイトル | ||||||
言語 | en | |||||
タイトル | Voltammetry of immobilized cytochrome c on novel binary self-assembled monolayers of thioctic acid and thioctic amide modified gold electrodes | |||||
言語 | ||||||
言語 | eng | |||||
資源タイプ | ||||||
資源 | http://purl.org/coar/resource_type/c_6501 | |||||
タイプ | journal article | |||||
著者 |
Ji, XP
× Ji, XP× Jin, BK× Jin, JY× Nakamura, T |
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信州大学研究者総覧へのリンク | ||||||
氏名 | Jin, JY | |||||
URL | http://soar-rd.shinshu-u.ac.jp/profile/ja.jUThymkV.html | |||||
出版者 | ||||||
出版者 | ELSEVIER SCIENCE SA | |||||
引用 | ||||||
内容記述タイプ | Other | |||||
内容記述 | JOURNAL OF ELECTROANALYTICAL CHEMISTRY. 590(2): 173-180 (2006) | |||||
書誌情報 |
JOURNAL OF ELECTROANALYTICAL CHEMISTRY 巻 590, 号 2, p. 173-180, 発行日 2006-05-15 |
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資源タイプ(コンテンツの種類) | ||||||
内容記述タイプ | Other | |||||
内容記述 | Article | |||||
ISSN | ||||||
収録物識別子タイプ | ISSN | |||||
収録物識別子 | 0022-0728 | |||||
書誌レコードID | ||||||
収録物識別子タイプ | NCID | |||||
収録物識別子 | AA10836527 | |||||
他の資源との関係:URI | ||||||
識別子タイプ | URI | |||||
関連識別子 | http://www.elsevier.com/wps/find/journaldescription.cws_home/504087/description#description | |||||
関連名称 | http://www.elsevier.com/wps/find/journaldescription.cws_home/504087/description#description | |||||
DOI | ||||||
識別子タイプ | DOI | |||||
関連識別子 | https://doi.org/10.1016/j.jelechem.2006.03.011 | |||||
関連名称 | 10.1016/j.jelechem.2006.03.011 | |||||
出版タイプ | ||||||
出版タイプ | AM | |||||
出版タイプResource | http://purl.org/coar/version/c_ab4af688f83e57aa | |||||
WoS | ||||||
表示名 | Web of Science | |||||
URL | http://gateway.isiknowledge.com/gateway/Gateway.cgi?&GWVersion=2&SrcAuth=ShinshuUniv&SrcApp=ShinshuUniv&DestLinkType=FullRecord&DestApp=WOS&KeyUT=000238304400008 |