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Through simple conformal coating, different weight of conductive PEDOT/PSS papers were fabricated and exhibited electromechanical actuation with stress generation controlled by low alternating applied voltage in ambient air. The dependence of electromechanical actuation on the weight of PEDOT/PSS and the frequency of the applied voltage are determined. The repeatability of the actuation is confirmed by generation of a stable stress more than 2000 times under ambient conditions. Furthermore, the PEDOT/PSS paper underwent intensive bending/unbending motion and showed a dependence on relative humidity. 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Through simple conformal coating, different weight of conductive PEDOT/PSS papers were fabricated and exhibited electromechanical actuation with stress generation controlled by low alternating applied voltage in ambient air. The dependence of electromechanical actuation on the weight of PEDOT/PSS and the frequency of the applied voltage are determined. The repeatability of the actuation is confirmed by generation of a stable stress more than 2000 times under ambient conditions. Furthermore, the PEDOT/PSS paper underwent intensive bending/unbending motion and showed a dependence on relative humidity. 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