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The internal tube wall of the negative curvature showed the higher adsorptivities for supercritical CH(4) and H(2) than the external tube wall of the positive curvature due to their interaction potential difference. Fine SWCNT bundles were prepared by the capillary force-aided drying treatment using toluene or methanol in order to produce the interstitial pore spaces having the strongest interaction potential for CH(4) or H(2); the bundled SWCNT showed the highest adsorptivity for supercritical CH(4) and H(2). 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