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  1. 080 繊維学部
  2. 0801 学術論文

Nanostructured RuO2 on MWCNTs: Efficient catalyst for transfer hydrogenation of carbonyl compounds and aerial oxidation of alcohols

http://hdl.handle.net/10091/17821
ceb1686c-de76-4ef3-b061-b716bb999863
名前 / ファイル ライセンス アクション
140_Nanostructured_RuO2_MWCNTs_Efficient_catalyst.pdf 140_Nanostructured_RuO2_MWCNTs_Efficient_catalyst.pdf (1.5 MB)
Item type 学術雑誌論文 / Journal Article(1)
公開日 2014-08-25
タイトル
言語 en
タイトル Nanostructured RuO2 on MWCNTs: Efficient catalyst for transfer hydrogenation of carbonyl compounds and aerial oxidation of alcohols
言語
言語 eng
キーワード
主題Scheme Other
主題 MWCNTs
キーワード
主題Scheme Other
主題 RuO2 nanostructures
キーワード
主題Scheme Other
主題 Dry synthesis
キーワード
主題Scheme Other
主題 Heterogeneous catalyst
キーワード
主題Scheme Other
主題 Transfer hydrogenation
キーワード
主題Scheme Other
主題 Aerial oxidation
資源タイプ
資源 http://purl.org/coar/resource_type/c_6501
タイプ journal article
著者 Gopiraman, M

× Gopiraman, M

WEKO 40338

Gopiraman, M

Search repository
Babu, S. Ganesh

× Babu, S. Ganesh

WEKO 40339

Babu, S. Ganesh

Search repository
Karvembu, R

× Karvembu, R

WEKO 40340

Karvembu, R

Search repository
Kim, I.S.

× Kim, I.S.

WEKO 40341

Kim, I.S.

Search repository
信州大学研究者総覧へのリンク
氏名 Kim, I.S.
URL http://soar-rd.shinshu-u.ac.jp/profile/ja.jNyCjFkV.html
出版者
出版者 ELSEVIER
引用
内容記述タイプ Other
内容記述 Applied Catalysis A. 484(22):84-96 (2014)
書誌情報 Applied Catalysis A

巻 484, 号 22, p. 84-96, 発行日 2014-08
抄録
内容記述タイプ Abstract
内容記述 Multiwall carbon nanotubes (MWCNTs)/ruthenium dioxide nanoparticles (RuO2NPs) composite was prepared by a straightforward ‘dry synthesis’ method. After being well characterized, the prepared composite was used as a nanocatalyst (RuO2/MWCNT) for the transfer hydrogenation of carbonyl compounds. The excellent adhesion of RuO2NPs on the anchoring sites of MWCNTs was confirmed by TEM and Raman analyses. The weight percentage (7.97 wt%) and the chemical state (+4) of Ru in RuO2/MWCNT was confirmed by EDS and XPS analyses, respectively. It was found that the RuO2/MWCNT has a higher specific surface area of 189.3 m2 g?1. Initially the reaction conditions were optimized and then the scope of the catalytic system was extended with a wide range of carbonyl compounds. The influence of the size of RuO2NPs on the transfer hydrogenation of carbonyl compounds was also studied. The RuO2/MWCNT is highly chemoselective, heterogeneous in nature, reusable and highly stable. Owing to the high stability of the used catalyst (u-RuO2/MWCNT), it was further calcinated at high temperature to obtain RuO2 nanorods (NRs) hybrid MWCNTs. Then the hybrid material was used as a catalyst (r-RuO2/MWCNT) for the aerial oxidation of alcohols and the result was found to be good.
資源タイプ(コンテンツの種類)
内容記述タイプ Other
内容記述 Article
ISSN
収録物識別子タイプ ISSN
収録物識別子 0926-860X
書誌レコードID
収録物識別子タイプ NCID
収録物識別子 AA10821202
DOI
関連識別子
識別子タイプ DOI
関連識別子 https://doi.org/10.1016/j.apcata.2014.06.032
関連名称
関連名称 10.1016/j.apcata.2014.06.032
権利
権利情報 Copyright© 2014 Elsevier B.V.
出版タイプ
出版タイプ AM
出版タイプResource http://purl.org/coar/version/c_ab4af688f83e57aa
WoS
表示名 Web of Science
URL http://gateway.isiknowledge.com/gateway/Gateway.cgi?&GWVersion=2&SrcAuth=ShinshuUniv&SrcApp=ShinshuUniv&DestLinkType=FullRecord&DestApp=WOS&KeyUT=000342476700012
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