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Nanostructured RuO2 on MWCNTs: Efficient catalyst for transfer hydrogenation of carbonyl compounds and aerial oxidation of alcohols
http://hdl.handle.net/10091/17821
http://hdl.handle.net/10091/17821ceb1686c-de76-4ef3-b061-b716bb999863
名前 / ファイル | ライセンス | アクション |
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140_Nanostructured_RuO2_MWCNTs_Efficient_catalyst.pdf (1.5 MB)
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Item type | 学術雑誌論文 / Journal Article(1) | |||||
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公開日 | 2014-08-25 | |||||
タイトル | ||||||
言語 | en | |||||
タイトル | Nanostructured RuO2 on MWCNTs: Efficient catalyst for transfer hydrogenation of carbonyl compounds and aerial oxidation of alcohols | |||||
言語 | ||||||
言語 | eng | |||||
DOI | ||||||
識別子タイプ | DOI | |||||
関連識別子 | https://doi.org/10.1016/j.apcata.2014.06.032 | |||||
関連名称 | 10.1016/j.apcata.2014.06.032 | |||||
キーワード | ||||||
主題 | MWCNTs, RuO2 nanostructures, Dry synthesis, Heterogeneous catalyst, Transfer hydrogenation, Aerial oxidation | |||||
資源タイプ | ||||||
資源 | http://purl.org/coar/resource_type/c_6501 | |||||
タイプ | journal article | |||||
著者 |
Gopiraman, M
× Gopiraman, M× Babu, S. Ganesh× Karvembu, R× Kim, I.S. |
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信州大学研究者総覧へのリンク | ||||||
氏名 | Kim, I.S. | |||||
URL | http://soar-rd.shinshu-u.ac.jp/profile/ja.jNyCjFkV.html | |||||
出版者 | ||||||
出版者 | ELSEVIER | |||||
引用 | ||||||
内容記述タイプ | Other | |||||
内容記述 | Applied Catalysis A. 484(22):84-96 (2014) | |||||
書誌情報 |
Applied Catalysis A 巻 484, 号 22, p. 84-96, 発行日 2014-08 |
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抄録 | ||||||
内容記述タイプ | Abstract | |||||
内容記述 | Multiwall carbon nanotubes (MWCNTs)/ruthenium dioxide nanoparticles (RuO2NPs) composite was prepared by a straightforward ‘dry synthesis’ method. After being well characterized, the prepared composite was used as a nanocatalyst (RuO2/MWCNT) for the transfer hydrogenation of carbonyl compounds. The excellent adhesion of RuO2NPs on the anchoring sites of MWCNTs was confirmed by TEM and Raman analyses. The weight percentage (7.97 wt%) and the chemical state (+4) of Ru in RuO2/MWCNT was confirmed by EDS and XPS analyses, respectively. It was found that the RuO2/MWCNT has a higher specific surface area of 189.3 m2 g?1. Initially the reaction conditions were optimized and then the scope of the catalytic system was extended with a wide range of carbonyl compounds. The influence of the size of RuO2NPs on the transfer hydrogenation of carbonyl compounds was also studied. The RuO2/MWCNT is highly chemoselective, heterogeneous in nature, reusable and highly stable. Owing to the high stability of the used catalyst (u-RuO2/MWCNT), it was further calcinated at high temperature to obtain RuO2 nanorods (NRs) hybrid MWCNTs. Then the hybrid material was used as a catalyst (r-RuO2/MWCNT) for the aerial oxidation of alcohols and the result was found to be good. | |||||
資源タイプ(コンテンツの種類) | ||||||
内容記述タイプ | Other | |||||
内容記述 | Article | |||||
ISSN | ||||||
収録物識別子タイプ | ISSN | |||||
収録物識別子 | 0926-860X | |||||
書誌レコードID | ||||||
収録物識別子タイプ | NCID | |||||
収録物識別子 | AA10821202 | |||||
権利 | ||||||
権利情報 | Copyright© 2014 Elsevier B.V. | |||||
出版タイプ | ||||||
出版タイプ | AM | |||||
出版タイプResource | http://purl.org/coar/version/c_ab4af688f83e57aa | |||||
WoS | ||||||
表示名 | Web of Science | |||||
URL | http://gateway.isiknowledge.com/gateway/Gateway.cgi?&GWVersion=2&SrcAuth=ShinshuUniv&SrcApp=ShinshuUniv&DestLinkType=FullRecord&DestApp=WOS&KeyUT=000342476700012 |