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The C-60/SiO2 powder was simply prepared by mixing a toluene solution of the C-60 fullerene with silica gel followed by evaporating the toluene. Irradiation by visible light (\u003e420 nm) of the methyl orange aqueous solution (25 mu M) in the presence of the C-60/SiO2 powder and ascorbic acid resulted in the decomposition of the methyl orange. These results showed that the degradation conversion reached 96% after a 25-min visible light irradiation. The reaction also occurred by the irradiation of sunlight. The reductive products of methyl orange, N,N-dimethyl-p-phenylenediamine and sulfanilic acid, were ascertained and monitored by liquid chromatography/mass spectrometry (LC/MS). The reaction did not occur in the dark and in the absence of C-60/SiO2 or ascorbic acid. The possible mechanism of the reaction is discussed. Furthermore, the C-60/SiO2 powder was applied to a continuous flow system for the photodecomposition of methyl orange. C-60/SiO2 powder was packed in a glass tube. 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Decomposition of methyl orange using C-60 fullerene adsorbed on silica gel as a photocatalyst via visible-light induced electron transfer
http://hdl.handle.net/10091/00018688
http://hdl.handle.net/10091/000186881e4f694e-06c3-48a9-8f39-53cdb260fb63
名前 / ファイル | ライセンス | アクション |
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Decomposition_of_methyl_orange_using.pdf (1.1 MB)
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Item type | 学術雑誌論文 / Journal Article(1) | |||||
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公開日 | 2016-03-23 | |||||
タイトル | ||||||
言語 | en | |||||
タイトル | Decomposition of methyl orange using C-60 fullerene adsorbed on silica gel as a photocatalyst via visible-light induced electron transfer | |||||
言語 | ||||||
言語 | eng | |||||
DOI | ||||||
識別子タイプ | DOI | |||||
関連識別子 | https://doi.org/10.1016/j.apcatb.2014.12.010 | |||||
関連名称 | 10.1016/j.apcatb.2014.12.010 | |||||
キーワード | ||||||
主題 | Fullerene, C-60 fullerene adsorbed on silica gel, Photoinduced electron-transfer, Visible light, Methyl orange | |||||
資源タイプ | ||||||
資源 | http://purl.org/coar/resource_type/c_6501 | |||||
タイプ | journal article | |||||
著者 |
Wakimoto, Ryo
× Wakimoto, Ryo× Kitamura, Tamako× Ito, Fuyu× Usami, Hisanao× Moriwaki, Hiroshi |
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信州大学研究者総覧へのリンク | ||||||
氏名 | Usami, Hisanao | |||||
URL | http://soar-rd.shinshu-u.ac.jp/profile/ja.uacFjekV.html | |||||
信州大学研究者総覧へのリンク | ||||||
氏名 | Moriwaki, Hiroshi | |||||
URL | http://soar-rd.shinshu-u.ac.jp/profile/ja.jCyFjFkV.html | |||||
出版者 | ||||||
出版者 | ELSEVIER SCIENCE BV | |||||
引用 | ||||||
内容記述タイプ | Other | |||||
内容記述 | APPLIED CATALYSIS B-ENVIRONMENTAL. 166:544-550 (2015) | |||||
書誌情報 |
APPLIED CATALYSIS B-ENVIRONMENTAL 巻 166, p. 544-550, 発行日 2015-05 |
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抄録 | ||||||
内容記述タイプ | Abstract | |||||
内容記述 | Visible-light induced electron transfer reactions of C60 fullerene adsorbed on silica gel (C60/SiO2 powder) to methyl orange in water have been studied. The C60/SiO2 powder was simply prepared by mixing a toluene solution of the C60 fullerene with silica gel followed by evaporating the toluene. Irradiation by visible light (>420 nm) of the methyl orange aqueous solution (25 μM) in the presence of the C60/SiO2 powder and ascorbic acid resulted in the decomposition of the methyl orange. These results showed that the degradation conversion reached 96% after a 25-min visible light irradiation. The reaction also occurred by the irradiation of sunlight. The reductive products of methyl orange, N,N-dimethyl-p-phenylenediamine and sulfanilic acid, were ascertained and monitored by liquid chromatography/mass spectrometry (LC/MS). The reaction did not occur in the dark and in the absence of C60/SiO2 or ascorbic acid. The possible mechanism of the reaction is discussed. Furthermore, the C60/SiO2 powder was applied to a continuous flow system for the photodecomposition of methyl orange. C60/SiO2 powder was packed in a glass tube. The methyl orange solution was pumped into the glass tube, and the tube was irradiated by visible light or sunlight. The continuous decomposition of methyl orange was achieved by this method. | |||||
資源タイプ(コンテンツの種類) | ||||||
内容記述タイプ | Other | |||||
内容記述 | Article | |||||
ISSN | ||||||
収録物識別子タイプ | ISSN | |||||
収録物識別子 | 0926-3373 | |||||
書誌レコードID | ||||||
収録物識別子タイプ | NCID | |||||
収録物識別子 | AA1082551X | |||||
権利 | ||||||
権利情報 | © 2015. This manuscript version is made available under the CC-BY-NC-ND 4.0 license http://creativecommons.org/licenses/by-nc-nd/4.0/ | |||||
出版タイプ | ||||||
出版タイプ | AM | |||||
出版タイプResource | http://purl.org/coar/version/c_ab4af688f83e57aa | |||||
WoS | ||||||
表示名 | Web of Science | |||||
URL | http://gateway.isiknowledge.com/gateway/Gateway.cgi?&GWVersion=2&SrcAuth=ShinshuUniv&SrcApp=ShinshuUniv&DestLinkType=FullRecord&DestApp=WOS&KeyUT=000348753400060 |