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  1. 060 工学部
  2. 0601 学術論文

Suppressing the effect of lithium dendritic growth by the addition of magnesium bis(trifluoromethanesulfonyl)amide

http://hdl.handle.net/10091/00021824
5510eb87-986d-4561-bd7b-dcf8ce3c8bcb
名前 / ファイル ライセンス アクション
16H06838_02.pdf 16H06838_02.pdf (3.2 MB)
16H06838_02_SupplementaryData.pdf 16H06838_02_SupplementaryData.pdf (3.5 MB)
Item type 学術雑誌論文 / Journal Article(1)
公開日 2020-01-30
タイトル
言語 en
タイトル Suppressing the effect of lithium dendritic growth by the addition of magnesium bis(trifluoromethanesulfonyl)amide
言語
言語 eng
資源タイプ
資源 http://purl.org/coar/resource_type/c_6501
タイプ journal article
著者 Shimizu, Masahiro

× Shimizu, Masahiro

WEKO 108860

Shimizu, Masahiro

Search repository
Umeki, Makoto

× Umeki, Makoto

WEKO 108861

Umeki, Makoto

Search repository
Arai, Susumu

× Arai, Susumu

WEKO 108862

Arai, Susumu

Search repository
信州大学研究者総覧へのリンク
氏名 Shimizu, Masahiro
URL http://soar-rd.shinshu-u.ac.jp/profile/ja.gCkVbUkh.html
信州大学研究者総覧へのリンク
氏名 Arai, Susumu
URL http://soar-rd.shinshu-u.ac.jp/profile/ja.jUyhbpkh.html
出版者
出版者 ROYAL SOC CHEMISTRY
引用
内容記述タイプ Other
内容記述 PHYSICAL CHEMISTRY CHEMICAL PHYSICS.20(2):1127-1133(2018)
書誌情報 PHYSICAL CHEMISTRY CHEMICAL PHYSICS

巻 20, 号 2, p. 1127-1133, 発行日 2017-12-05
抄録
内容記述タイプ Abstract
内容記述 Practical applications of Li-S and Li-air batteries require the morphology of the Li metal negative electrode during charge/discharge (i.e., Li-deposition/dissolution) cycling to be precisely controlled. Herein, we used magnesium bis(trifluoromethanesulfonyl)amide [Mg(TFSA)(2)] as an electrolyte additive to suppress the growth of Li dendrites, utilizing the occurrence of an alloying reaction between the initially substrate-deposited Mg and the subsequently deposited Li. Notably, no metallic Mg formation and no change in Li deposition morphology were observed at an electrolyte composition of 0.1 M Mg(TFSA)(2) + 0.9 M LiTFSA/triglyme, irrespective of the applied potential. In contrast, increasing the Mg salt concentration to 0.5 M resulted in the deposition of interconnected granules, reflecting a dramatic morphology improvement. X-ray diffraction analysis revealed the occurrence of the abovementioned alloying, which finally afforded a deposit composition of Li0.9Mg0.1 via the formation of an intermediate Li0.14Mg0.86 phase. Importantly, the deposits obtained under various applied potentials were relatively smooth, with no needle-like morphology observed.
資源タイプ(コンテンツの種類)
内容記述タイプ Other
内容記述 Article
ISSN
収録物識別子タイプ ISSN
収録物識別子 1463-9076
書誌レコードID
収録物識別子タイプ NCID
収録物識別子 AA11301773
DOI
関連識別子
識別子タイプ DOI
関連識別子 https://doi.org/10.1039/c7cp06057b
関連名称
関連名称 10.1039/c7cp06057b
出版タイプ
出版タイプ AM
出版タイプResource http://purl.org/coar/version/c_ab4af688f83e57aa
WoS
表示名 Web of Science
URL http://gateway.isiknowledge.com/gateway/Gateway.cgi?&GWVersion=2&SrcAuth=ShinshuUniv&SrcApp=ShinshuUniv&DestLinkType=FullRecord&DestApp=WOS&KeyUT=000419219700044
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